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Quantifying sources of methane using light alkanes in the Los Angeles basin, California

Journal of Geophysical Research: Atmospheres, vol.118 no.10 pp.4974-4990, 27/05/2013

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Resource information:
Resource IDpeischl2013
Resource titleQuantifying sources of methane using light alkanes in the Los Angeles basin, California
Author(s)J. Peischl, T.B. Ryerson, J. Brioude, K.C. Aikin, A.E. Andrews, E. Atlas, D. Blake, B.C. Daube, J.A. de Gouw, E. Dlugokencky, G.J. Frost, D.R. Gentner, J.B. Gilman, A.H. Goldstein, R.A. Harley, J.S. Holloway, J. Kofler, W.C. Kuster, P.M. Lang, P.C. Novelli, G.W. Santoni, M. Trainer, S.C. Wofsy, D.D. Parrish
Publication/ sourceJournal of Geophysical Research: Atmospheres, vol.118 no.10 pp.4974-4990
Date published27/05/2013
Summary text/ abstractMethane (CH4), carbon dioxide (CO2), carbon monoxide (CO), and C2-C5 alkanes were measured throughout the Los Angeles (L.A.) basin in May and June 2010. We use these data to show that the emission ratios of CH4/CO and CH4/CO2 in the L.A. basin are larger than expected from population-apportioned bottom-up state inventories, consistent with previously published work. We use experimentally determined CH4/CO and CH4/CO2 emission ratios in combination with annual State of California CO and CO2 inventories to derive a yearly emission rate of CH4 to the L.A. basin. We further use the airborne measurements to directly derive CH4 emission rates from dairy operations in Chino, and from the two largest landfills in the L.A. basin, and show these sources are accurately represented in the California Air Resources Board greenhouse gas inventory for CH4. We then use measurements of C2-C5 alkanes to quantify the relative contribution of other CH4 sources in the L.A. basin, with results differing from those of previous studies. The atmospheric data are consistent with the majority of CH4 emissions in the region coming from fugitive losses from natural gas in pipelines and urban distribution systems and/or geologic seeps, as well as landfills and dairies. The local oil and gas industry also provides a significant source of CH4 in the area. The addition of CH4 emissions from natural gas pipelines and urban distribution systems and/or geologic seeps and from the local oil and gas industry is sufficient to account for the differences between the top-down and bottom-up CH4 inventories identified in previously published work.
Library categoriesClimate Change, Extr. Energy Climate
Added to Free Range Library17/05/2014
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